Radiation-responsive apparatus



July 8', 1958 c. GooDMAN 2,842,695

RADIATION-RESPONSIVE APPARATUS Filed may 1v. 1954 INTEGRATO?? GRECORDER CLARK GOODMAN BY WMI/U` HIS ATTORNEY the. target'. obviously this control system may. not'providefthedesired` A V lf'constant neutron output of the generator, andza. monitorresponsive vto'the neutron output of the.` generator may bebettersuited for maintaining; alconstant neutronV in.

2,842,695V f nAnrA'rIoN-Rnsronsivni APPARATUS.`

Clark Goodman, Boston, 'Massa assigner, by ,mesne assignments, to Schlumberger yWell Surveying'Corporas tion, Houstomv'lex., a corporation of Texas;

Application Mayr?, 1954, serial Nd. 436,139' v 7 Claims. (Ci: 313;'6'1) Although useful and of thertype including a generator of high energy y neutrons for irradiating earthv formations traversed by the boreholeand a detector for observing a resulting nuclear phenomenon.. For convenience, the invention will bede'scribed as embodied Yin `a typical system of this general 'character which may bek employed for logging the earth formations. Y f

Inorderto interpret the,secondaryradiations observed i' i ,whi1elogging with afgenerator'of highenergy neutrons,`

fit may: be desirable tomaintain a source intensity.

constant orv known Oneprior control system for; regulatingneutron, output is intended for usewith a generator whereinparticles-are i 'acceleratedir'ra beam toward `a target: Such asystem` is responsivetor and adjusts the beam'y of particlestin such.-

a manner as to maintaina constant current incidention Since the target Ymay become:y depleted,

tensity throughout an entire logging run.,

'A`conventional counter used in drillholedogging is responsive primarily to neutrons ofthermal energy?v level.-

' Sin'cethe borehole into which the.` logging zapparatusj .is lowered usually isl viilled with a drilling 'mudrinfwhichno neutrons 'may be slowed down; this detectorishndesir'- ably `sensitive to thev mud surrounding-the logging appar.-

ratus.V Moreover, some of. the earthformations may in a wide variety offapplication's, a Y neutrondetector in accordance with the present invention is ideally suited for use in apparatusv adapted to be passed through a well or borehole drilled into-the earth,

'Thisinvention relates to radiationresponsive apparatus 15 and,` more particularly, pertains to anew and improved'V neutron-- detector for derivingr indications of incident Y y neutronshaving anenergy'greater than va selected energy f' ice,

enter into reactions with incident neutrons. tofproduce` charged particlesconduciveto ionization in the chamber.

These charged particles are emitted with alrinetic energy, f

Ep, essentiallyequal. to. the sum,` ofthe incident neutronVVV energy, En, and the nuclear energy change, Q, ofthe reaction, i. e. EpEn-l-Q. In accordancewith the present invention a Qvis selected of negative value and suf-L ficiently lessin absolute magnitude than En ,to makelp.

a few million electron volts, for-[example Inthis way` the, ionization pulses vproducedby the charged particles are easily detectedfabove: background, radiations.

no greater than the selected energy level so, that there.

vis substantially no response to incident. neutrons having an energy below the selected level.

The y novel features A/of thefpresent inventionjare. set y forth with particularityinthe appended claims.y -The present invention,.both as to itsorganization and mannerk beflined with one or more: strings of metallicfcasingg o of operation, together with further-objectsand advantages Fig. 2 is: a. sectional view-taken alongthe line. 2`-Z of i Fig. l. v Y

In Fig.

the present inventionf isfyshown disposedfl in aborehole` l0; traversing4 kva pluralitypf-.earth formations 11. `1Bore.-, Y I

hole lt) usually.. containsashydrogenous drillinggliquide 12, such` vas a water basexor oil-'base mud; and'jit-may Y (not shown), ornit mayybe uncasedas illustratechf Y -The neutron wellY logging.;apparatus-maycomprise a pressure resistant 'housinggl-fsuspended; inthe borehole by means-.ofV an armored cable 14.1which,VV in connection' Y with a winch (not, shown) located .at tl1ef surfacegov the f boreholefin'the customary mannen Y Cable14 also includesna pluralitylofg insulated?con@ k ductors 15, 16 and;.17K andashield.- litflorl connecting` surfaceequipment.withgapparatuswithin housingll'.; VOli i containvwater or oilz in which;neutrons may be slowed..

down and the output of this detector represents thisf charf lacteristic of the earth' vformations,which vis undesirable in monitoring the neutron source.

natingcurrent 159fto. ya, medium voltagegpower- ;supp ly120 l and via -a voltage -control circuit,v 21to1be described more;

fully hereinaftenandfa conductor-22 to ahigh voltage 'Y power; supply 23. Y n

The power supplies 20A-ausiliareradapted to energize:l a neutron generator 24 which maybe of any cornvenf tional type including an ionsource-ZS wherein deuterium Itis, `therefore, an object ofy the' present Y"invention to provide a new'and improved neutron detector which is notsubject to the foregoing deficiencies'of prior'arrange# ments.

Another object of the present invention'v is to, provide a new and improved;neutromdetector forderiving `indic'ationsbf incident neutrons fhavingan energy greater than a` selected level,"v and' which is" substantially unresponsive to 'neutronsy having `anenergy-k below the selected level.'V

A' neutron-responsive deviceA embodying thez'present` invention is vadaptedito deriveY indications of'ffincidentl neutronsvhaving an energy greater than, afselectedfl'evel and'is comprised ofla chamber in which iom'zation'may u pecar.' The' chamber encloses a substance adapted' to Y generatorzzl, a detector zembodying tliepresentinven.

ions are derived andan acceleratinggapZ `for acceleratj ing such ionstoward'a deuteriunror ,tritium target}to.

a velocity at` which neutronfproducing reactionsj- .may p occur. For example, vas illustrated'in the dr` 'awing, ion

source 25 maybe ofthe specific type kdisclosedinthe j copending application ofJ-JZTI Dewan, iiled April9`, 1952]f `bearing the Serial vNumber 28 1',3 78-and assigned to the same assigneeas the present invention; Power supplyy 20 is arranged in themanner describedjin 'the Dewan applicati/onto energize ion source 25., Acceleratinggap 26' maynbevsimilar, to any one of'the varieties disclosed;r in the copending application off Waynel R. Arnold, filed:

assigned to the same assignee as the present invention.

, In, order-1 tov control tlieinel-ltroijh I f f* 2,842,695 Fatented July 8,.A 1 958,

In." i

,Y otherwords, the reactionsmay exhibita nuclear energychange of negative sense: and otY an, absolute. magnitude'. Y

1 ofL theA drawing. thejneutronjwell: logging` Vapparatus providedlwitha neutron detector-embodying tion, and to be described in detail hereinafter, is disposed in housing 13 in the general vicinity of the target portion of accelerating gap 26. One output lead of detector 27 is grounded to housing 13 and the remaining output lead is connected by a lead 28 to a coupling condenser 29, in turn, connected to a conventional pulse amplifier and integrator unit 30. The necessary voltage for detector 27 is derived from power supply 2@ over a decoupling resistor 31.

The output potential of unit 30, which is representative of a characteristic of the generated neutron tlux, such as counts per unit time, is applied to the input circuit of voltage control circuit 21 over leads 32.

Elements 20, 21, 23 and 3) may be of conventional construction, or of the types described in the aforementioned Arnold application. As there stated, control circuit 21 may include a magneticamplilier connected in a servo-circuit which compares the potential from amplitier-integrator 30 with a reference potential to derive a control effect. This control effect may be the adjustment of the value of an impedance effectively connected between leads and 22. Accordingly, the potential which energizes high voltage power supply 23 is dependent upon the generated neutron iux.

To obtain a log, for example, of the resulting gamma radiation, a radioactivity responsive device or detector 33 is supported at the lower end of housing 13 below a shield plate 34 employed to shield the detector from radiation emanating from generator 24. Detector 33 may be a suitably energized Geiger-Mueller tube coupled to an amplier 35 having its output circuit connected to lead 17 and housing 13. The output of amplier 35 is derived at the surface of the earth by connections from lead 17 and shield 18 to an integrator and recorder unit 36. Unit 36, for example, may comprise a capacitor for deriving a potential representing the number of pulses applied per unit time and a recording voltmeter to which this potential is applied. The recording medium of the voltmeter is displaced in a customary manner in synchronism with movement of housing 13 through borehole 10 so that a continuous log may be obtained.

Turning now to the details of neutron detector 27 embodying the present invention, as shown in Fig. 2, the detector is comprised of a housing 37 constructed of an electrically conductive material such as steel. The detector is provided with a conductive, central electrode 38 and is lined with a substance 39 responsive to fast neutrons. For example, tantalum oxide may be employed wherein the oxygen is 99.76% of atomic weight 16. The oxygen in layer 39 is adapted to enter into reactions with incident neutrons to produce charged particles, such as protons. These charged particles are emitted with a kinetic energy, Ep, essentially equal to the sum of the incident neutron energy, En, and the nuclear energy change, Q, of the reaction. This relationship may be expressed as follows:

EpEn-ro (1) In accordance with the present invention a Q is selected of negative value and sufficiently less in absolute magnitude than En so that Ep becomes a few million electron volts to satisfy Equation 1 above. In other words, these reactions exhibit a nuclear energy change of negative sense and of an absolute magnitude such that these reactions are not produced by the neutrons returned toward housing 13 from formations 11 and drilling mud 12. In this illustrative example, the nuclear energy change or Q is minus 9.24 million electron volts (m. e. v.). The space between electrode 38 and layer 39 of the detector is filled to a pressure of a few centimeters of mercury with an ionizable gas, such as argon, adapted to become ionized in the presence of the protons derived in layer 39, but of large enough atomic weight to give negligible -ionization when struck by a fast neutron. Connections to detector 27 are completed by a lead be- 4 tween housings 13 and 37 and by extending lead 28 to electrode 38.

In operation, housing 13 is lowered into borehole 10 prior to the closing of a control switch (not shown). This switch connects source 19 to leads 15 and 16 and thus neutron generator 24 is energized by power supplies 2G and 23. Deuterium ions are derived in ion source 25 and some of these enter accelerating gap 26. Accord ingly, highly accelerated positive deuteriurn ions react with tritium in the target portion of the accelerating gap and neutrons at an energy level of 14 m. e. v. are generated.

High energy neutrons emanating from generator 24 irradiate earth formations 11 and some of the resulting f nuclear radiation is incident on Geiger-Mueller tube 33.

Detector 33 responds to gamma radiation and its output is ampliiied in amplifier 35 and supplied to the integrator and recorder unit 36 so that a neutron-gamma ray log is obtained. Such a log features information regarding the earth formations traversed by the borehole as enumerated in detailV Vin the copending application of Clark Goodman, led March 1l, 1952, bearing Serial Number 275,932 and assigned to the same assignee as the present invention.

A small fraction of the 14 m. e. v. neutrons emanating from generator 24 arriving at detector 27, traverse housing 37 and enter layer 39. Some of these neutrons enter into reactions with the oxygen of layer 39 and the resulting protons cause ionization of the argon within the detector. Each time ionization occurs, a pulse is developed and the resulting pulses are amplified and integrated in stage 3d to develop a control potential which is supplied to voltage control circuit 21.

If the neutron tlux on detector 27 increases, the nurnber of counts per second increases, and the voltage control circuit reduces the voltage supplied to high voltage power supply 23. Accordingly, a lower voltage is applied to accelerating gap 26, thereby decreasing the neutron liux. Conversely, a decrease in the neutron tlux causes an increase in the high voltage supplied to the accelerating gap. In this way, the neutron yield remains substantially constant over a wide variety of operating conditions.

Since the reaction between the oxygen and the neutrons involves a high negative Q, scattered neutrons of low energy do not react to any appreciable extent. However, the cross section of the reaction and the energy of the resulting protons are ideally suited for monitoring high energy neutrons.

Because the cross section of the neutron-oxygen reaction is `only moderate, the counter may be located directly adjacent the target of accelerating gap 26 without obtaining unduly high counting rates. This close spatial relationship may be employed, even though the neutron yield may be las high as 109 0r 1010 neutrons per second.

It is evident, therefore, that a neutron detector constructed in `accordance with the present invention is adapted to derive indications ofincident neutrons having an energy greater than a selected energy level, and is substantially unresponsive to neutrons whose energy is lower than this level. Accordingly, the detector is not subject to the deciencies of various prior arrangements.

If desired, instead of automatic control, manual control may lbe provided. In this connection, the output of unit 30 is supplied to an indicator (not shown) at the surface of the earth instead of to control circuit 21. A suitable arrangement of a battery and potentiometer (not shown) may be connected to leads 32 for producing a control signal to adjust circuit 21.

The detector may, of course, be lled with other kinds of gases. For example, krypton and xenon may be employed.

.If desired, ineplace of steel housing 37 and tantalum oxide layer39, an aluminum housing may be utilized on i the insideof Whichfis a thin surface layer `of aluminum oxide.

Alternatively, instead of lining the' housing 37 withl a material responsive to fast' neutrons, the proportional counter may be lled with a gas, such' as oxygemadapted to' enter into reactions with neutrons wherein the nu clear energy change is of negative sense and of the desired labsolute magnitude.

Althoughzoxygen has been suggested hereinbefore as one of the materials adaptedto react with incident neutrons above a selected energy level, any of the following substances may be suitably employed:

Substance Q., Reaction 1n. e. v.

Neon (as gas) 1. 5 Neim) Phosphorus (as element or compounds) 1. 3 Plmp) Sulfur (as element or compounds). 0. 9 Krap) Thorium (as element or compounds) 1.0 Thmtmf) These substances are especially 'suited for monitoring the output of a generator which derives neutrons at an Aen ergy in the neighborhood of 3 m. e. v., such as where deuterium-deuterium reactions are involved.

'While particular embodiments of the present invention have been described, it is apparent that changes and modiications may be made without departing from this invention in its broader aspects,rand therefore the aim in the appended claims is to cover all such changes and I modications as fall within Vthe true spirit and scope of this invention.

I claim: 1. A neutron-responsive device `for deriving indications e of incident neutrons having an energy at least equal toa selected energy level substantially tothe exclusion of neutrons having an energy smaller than said selected energy level comprising a chamber wherein ionization may occur, and a substance enclosed by said chamber and.A

adapted to'enter into reactions with incident neutrons to producecharged particles conducive to said ionization,

said reactions exhibiting a nuclear energy change of neg ative sense and of an absolute magnitude substantially equal to said selected energy level.

2;'A neutron-responsive device for Vderiving indications of incident neutrons having an energy at least equal to a lselected energy level substantially to the exclusion y o fvneutrons'having an energy smaller than said selected energy level comprising a housing having an inner surface, an ionizable-gas enclosed by said housing, and a VVlayer of material covering said inner surface of said housing, at least, in part, and adapted to enter into reactions with incident neutrons to produce charged particles conducive to ionization ofvsaid gas, said reactions exhibiting a nuclear energy change of` negative sense and of an absolute magnitude substantially equal to said selected er1-A ergy level. 1

3. A neutron-responsive device ,for deriving indications of incident neutrons having an energy at least equal to a selected energy-level substantially to thev exclusion yofrneutrons having an energy smallerV than said` selected energyl level comprising a .housing having an inner survface, an ionizable Vgas enclosed by said housing, and a layer ofrmaterial included in said innersurface ofsaid housingl and adapted to enter into reactions with incito ionization of said gas, said reactions exhibiting a nu-V clear energy change of negative sense, and of an absolute magnitude substantially equal to said selected l energy level.

4. A neutron-responsive device for deriving indications -of incident neutrons having an energy at least equal to a selected energy level substantially to the exclusion of neutrons having an energy smaller than said selected energy level comprising a chamber, and an ionizable gas enclosed by said chamber and adapted to enter into reactions with incident neutrons to produce charged particles conductive to ionization, said reactions exhibiting a nuclear energy change of negative sense and ,of an absolute magnitudesubstantially-equal to said selected energy level.

5. A neutron-responsive device for deriving indications of incident neutrons having an energy at least equal to a selected energy level substantially to the'exclusion of neutrons having an energy smaller than said' selected energy level comprising a material defining ,a lchamber and adapted to enter into reactions with incident neutrons to produce charged particles, said reactions exhibiting a energy level comprising a chamber whereink ionization n may occur, and a substance enclosed by said chamber and adapted to enter into reactions with incident neutrons having an energy En to produce `charged particles having an energy Ep conducive to ionization of said gas,-

the relationship of En to Ep being expressed as follows:y EpEn-l-Q where Q is the nuclear energy change of said reactions,

and has negative value and an absolute magnitude substantially-equal to said selected energy level.

7. A radiation-responsive device rforV deriving indications of incident neutrons having an energy at least equal to a selected energy level substantially to the exclusion of neutrons having an energy smaller than Vsaid selected energy level comprising a chamber wherein ionization may occur, and a substance including oxygen enclosed by said chamber and adapted to enter into endothermic reactions with incident neutrons to produce charged particles conducive to said ionization.

References Cited inthe le of this patent UNITED STATES PATENTS OTHER REFERENCES f Li et ai.: Physica Review, v01. s3, pp.`r S12-'515 (1951 Kaumann et Jal. Jair. 20,1942 

